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Confinement‐Locking Strategy Enables Ionogels With Remarkable Mechanical Robustness and Fatigue Resistance
A confinement-locking strategy is developed to fabricate mechanically robust and fatigue-resistant phase-separated ionogels: part of soft segments are confined in hard domains to buffer stress and facilitate the reorganization of hydrogen-bonding assemblies, while IL is confined in soft phases to eliminate interference with hard segments and enhance the stability of hydrogen-bonding networks.
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